one time cheap molds = plaster
for bigger parts use wood and burlap backing on the other side
donot try to go too thin it will crack
and wax it heavily
for low production fiberglass itself is hard to beat as a mold material
now the buck the mold is made from [ the shape your are molding from ie the ''model part'']
can be anything plaster again clay wax urethane foam cardboard balsa or other wood ect
BUT a VERY GOOD SURFACE is needed to get a ultra smooth wax coat on a sealing layer [ paint ] if the material is porous
a good book on fiberglass boat building is a good starting point
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Question wonder and be wierd
are you kind?